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Photoinduced electron transfer in semiconductor–clay binary nanosheet colloids controlled by clay particles as a turnout switch
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10332328.pdf (3.6 MB)
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Item type | 学術雑誌論文 = Journal Article(1) | |||||||||||||||||||||||
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公開日 | 2021-03-10 | |||||||||||||||||||||||
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資源タイプ識別子 | http://purl.org/coar/resource_type/c_6501 | |||||||||||||||||||||||
資源タイプ | journal article | |||||||||||||||||||||||
タイトル | ||||||||||||||||||||||||
言語 | en | |||||||||||||||||||||||
タイトル | Photoinduced electron transfer in semiconductor–clay binary nanosheet colloids controlled by clay particles as a turnout switch | |||||||||||||||||||||||
言語 | ||||||||||||||||||||||||
言語 | eng | |||||||||||||||||||||||
著者 |
中戸, 晃之
× 中戸, 晃之
WEKO
28679
× Terada, Shinya× Ishiku, Tatsuya× Abe, Shungo× Kamimura, Sunao× 毛利, 恵美子
WEKO
14134
× 横野, 照尚
WEKO
6794
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抄録 | ||||||||||||||||||||||||
内容記述タイプ | Abstract | |||||||||||||||||||||||
内容記述 | Although semiconductor photocatalysis has been investigated actively for a long time, control of dark processes successive to electron transfer from photocatalysts is almost unexplored compared with designing photocatalysts themselves. The present study proposes employment of clay particles as for controlling the dark processes independently of semiconductor photocatalyst particles. We employed niobate–clay binary nanosheet colloids, where colloidal niobate and clay nanosheets are spatially separated at a micrometer level. Niobate nanosheets worked as the semiconductor photocatalyst that released electrons upon UV excitation, and clay nanosheets worked as the turnout switch of the released electrons to determine their destination. When methylviologen (MV2+) molecules that accept the electrons released from niobate were adsorbed on clay nanosheets, reduction of MV2+ predominantly occurred, and hydrogen was little evolved from the colloid. When Pt nanoparticles were deposited on clay nanosheets, photocatalytic hydrogen evolution occurred because Pt loaded on the clay nanoparticles played a role of cocatalyst. When MV2+ and Pt were co-loaded on clay nanosheets, both of MV2+ reduction and hydrogen evolution occurred competitively. The photocatalytic hydrogen evolution carried out by stirring the colloid sample was worse than that conducted without stirring, which indicated positive contribution of the spatial separation of photocatalytic niobate and cocatalytic clay nanosheets. | |||||||||||||||||||||||
書誌情報 |
Applied Catalysis B: Environmental 巻 241, p. 499-505, 発行日 2018-09-18 |
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出版者 | Elsevier | |||||||||||||||||||||||
DOI | ||||||||||||||||||||||||
関連タイプ | isVersionOf | |||||||||||||||||||||||
識別子タイプ | DOI | |||||||||||||||||||||||
関連識別子 | https://doi.org/10.1016/j.apcatb.2018.09.047 | |||||||||||||||||||||||
日本十進分類法 | ||||||||||||||||||||||||
主題Scheme | NDC | |||||||||||||||||||||||
主題 | 549 | |||||||||||||||||||||||
ISSN | ||||||||||||||||||||||||
収録物識別子タイプ | PISSN | |||||||||||||||||||||||
収録物識別子 | 0926-3373 | |||||||||||||||||||||||
ISSN | ||||||||||||||||||||||||
収録物識別子タイプ | EISSN | |||||||||||||||||||||||
収録物識別子 | 1873-3883 | |||||||||||||||||||||||
著作権関連情報 | ||||||||||||||||||||||||
権利情報 | Copyright (c) 2018 Elsevier B.V. All rights reserved. | |||||||||||||||||||||||
キーワード | ||||||||||||||||||||||||
主題Scheme | Other | |||||||||||||||||||||||
主題 | Nanosheet colloid | |||||||||||||||||||||||
キーワード | ||||||||||||||||||||||||
主題Scheme | Other | |||||||||||||||||||||||
主題 | Phase separation | |||||||||||||||||||||||
キーワード | ||||||||||||||||||||||||
主題Scheme | Other | |||||||||||||||||||||||
主題 | Photocatalytic hydrogen evolution | |||||||||||||||||||||||
キーワード | ||||||||||||||||||||||||
主題Scheme | Other | |||||||||||||||||||||||
主題 | Photoinduced electron transfer | |||||||||||||||||||||||
出版タイプ | ||||||||||||||||||||||||
出版タイプ | AM | |||||||||||||||||||||||
出版タイプResource | http://purl.org/coar/version/c_ab4af688f83e57aa | |||||||||||||||||||||||
査読の有無 | ||||||||||||||||||||||||
値 | yes | |||||||||||||||||||||||
研究者情報 | ||||||||||||||||||||||||
https://hyokadb02.jimu.kyutech.ac.jp/html/100000325_ja.html | ||||||||||||||||||||||||
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10332328 | ||||||||||||||||||||||||
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8568 | ||||||||||||||||||||||||
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内容記述タイプ | Other | |||||||||||||||||||||||
内容記述 | Journal Article | |||||||||||||||||||||||
著者別名 | ||||||||||||||||||||||||
姓名 | Nakato, Teruyuki | |||||||||||||||||||||||
言語 | en | |||||||||||||||||||||||
姓名 | 中戸, 晃之 | |||||||||||||||||||||||
言語 | ja | |||||||||||||||||||||||
姓名 | ナカト, テルユキ | |||||||||||||||||||||||
言語 | ja-Kana | |||||||||||||||||||||||
著者別名 | ||||||||||||||||||||||||
姓名 | Terada, S. | |||||||||||||||||||||||
著者別名 | ||||||||||||||||||||||||
姓名 | Ishiku, T. | |||||||||||||||||||||||
著者別名 | ||||||||||||||||||||||||
姓名 | Abe, S. | |||||||||||||||||||||||
著者別名 | ||||||||||||||||||||||||
姓名 | Kamimura, S. | |||||||||||||||||||||||
著者別名 | ||||||||||||||||||||||||
姓名 | Mouri, Emiko | |||||||||||||||||||||||
言語 | en | |||||||||||||||||||||||
姓名 | 毛利, 恵美子 | |||||||||||||||||||||||
言語 | ja | |||||||||||||||||||||||
姓名 | モウリ, エミコ | |||||||||||||||||||||||
言語 | ja-Kana | |||||||||||||||||||||||
著者別名 | ||||||||||||||||||||||||
姓名 | Ohno, Teruhisa | |||||||||||||||||||||||
言語 | en | |||||||||||||||||||||||
姓名 | 横野, 照尚 | |||||||||||||||||||||||
言語 | ja | |||||||||||||||||||||||
姓名 | オウノ, テルヒサ | |||||||||||||||||||||||
言語 | ja-Kana | |||||||||||||||||||||||
著者所属 | ||||||||||||||||||||||||
Department of Applied Chemistry, Kyushu Institute of Technology, 1-1 Sensui-cho, Tobata-ku, Kitakyushu, Fukuoka 804-8550, Japan, Strategic Research Unit for Innovative Multiscale Materials, Kyushu Institute of Technology, 1-1 Sensui-cho, Tobata-ku, Kitakyushu, Fukuoka 804-8550, Japan | ||||||||||||||||||||||||
著者所属 | ||||||||||||||||||||||||
Department of Applied Chemistry, Kyushu Institute of Technology, 1-1 Sensui-cho, Tobata-ku, Kitakyushu, Fukuoka 804-8550, Japan | ||||||||||||||||||||||||
著者所属 | ||||||||||||||||||||||||
Department of Applied Chemistry, Kyushu Institute of Technology, 1-1 Sensui-cho, Tobata-ku, Kitakyushu, Fukuoka 804-8550, Japan | ||||||||||||||||||||||||
著者所属 | ||||||||||||||||||||||||
Department of Applied Chemistry, Kyushu Institute of Technology, 1-1 Sensui-cho, Tobata-ku, Kitakyushu, Fukuoka 804-8550, Japan | ||||||||||||||||||||||||
著者所属 | ||||||||||||||||||||||||
Department of Applied Chemistry, Kyushu Institute of Technology, 1-1 Sensui-cho, Tobata-ku, Kitakyushu, Fukuoka 804-8550, Japan | ||||||||||||||||||||||||
著者所属 | ||||||||||||||||||||||||
Department of Applied Chemistry, Kyushu Institute of Technology, 1-1 Sensui-cho, Tobata-ku, Kitakyushu, Fukuoka 804-8550, Japan, Strategic Research Unit for Innovative Multiscale Materials, Kyushu Institute of Technology, 1-1 Sensui-cho, Tobata-ku, Kitakyushu, Fukuoka 804-8550, Japan | ||||||||||||||||||||||||
著者所属 | ||||||||||||||||||||||||
Department of Applied Chemistry, Kyushu Institute of Technology, 1-1 Sensui-cho, Tobata-ku, Kitakyushu, Fukuoka 804-8550, Japan, Strategic Research Unit for Innovative Multiscale Materials, Kyushu Institute of Technology, 1-1 Sensui-cho, Tobata-ku, Kitakyushu, Fukuoka 804-8550, Japan |