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Angular distributions of H-induced HD and D2 desorptions from the Si(100) surfaces
http://hdl.handle.net/10228/358
http://hdl.handle.net/10228/35856d192e9-1fd6-46cc-a07e-97bc59212c48
名前 / ファイル | ライセンス | アクション |
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1.2163339.pdf (305.7 kB)
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Item type | 学術雑誌論文 = Journal Article(1) | |||||
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公開日 | 2007-11-19 | |||||
資源タイプ | ||||||
資源タイプ識別子 | http://purl.org/coar/resource_type/c_6501 | |||||
資源タイプ | journal article | |||||
タイトル | ||||||
言語 | ja | |||||
タイトル | Angular distributions of H-induced HD and D2 desorptions from the Si(100) surfaces | |||||
言語 | ||||||
言語 | eng | |||||
著者 |
稲永, 征司
× 稲永, 征司× Kiyonaga, T.× Rahman, F.× Khanom, F.× 並木, 章× Lee, J. |
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抄録 | ||||||
内容記述タイプ | Abstract | |||||
内容記述 | We measured angular distributions of HD and D2 molecules desorbed via the reactions H+D/Si 100 →H+D/Si(100) → HD [abstraction (ABS)] and H+D/Si(100) →D2 [adsorption-induced-desorption (AID)], respectively. It was found that the angular distribution of HD molecules desorbed along ABS is broader than that of D2 molecules desorbed along AID, i.e., the former could be fit withcos2.0±0.2 θ, while the latter with cos5.0±0.5 θ. This difference of the angular distributions between the two reaction paths suggests that their dynamic mechanisms are different. The observed cos2 θ distribution for the ABS reaction was reproduced by the classical trajectory calculations over the London-Eyring-Polanyi-Sato potential-energy surfaces. The simulation suggests that the HD desorption along the ABS path takes place along the direction of Si–D bonds, but the apparent angular distribution is comprised of multiple components reflecting the different orientations of D-occupied Si dimers in the (2×1) and (1×2) double domain structures. | |||||
言語 | en | |||||
書誌情報 |
en : Journal of Chemical Physics 巻 124, 号 5, p. 054715-1-054715-6, 発行日 2006-02-07 |
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出版社 | ||||||
言語 | en | |||||
出版者 | American Institute of Physics | |||||
DOI | ||||||
関連タイプ | isIdenticalTo | |||||
識別子タイプ | DOI | |||||
関連識別子 | https://doi.org/10.1063/1.2163339 | |||||
CRID | ||||||
関連タイプ | isIdenticalTo | |||||
識別子タイプ | URI | |||||
関連識別子 | https://cir.nii.ac.jp/crid/1050001338909645824 | |||||
日本十進分類法 | ||||||
主題Scheme | NDC | |||||
主題 | 435 | |||||
NCID | ||||||
収録物識別子タイプ | NCID | |||||
収録物識別子 | AA00694991 | |||||
ISSN | ||||||
収録物識別子タイプ | EISSN | |||||
収録物識別子 | 1089-7690 | |||||
ISSN | ||||||
収録物識別子タイプ | PISSN | |||||
収録物識別子 | 0021-9606 | |||||
著作権関連情報 | ||||||
権利情報 | Copyright © 2006 American Institute of Physics | |||||
キーワード | ||||||
主題Scheme | Other | |||||
主題 | hydrogen compounds | |||||
キーワード | ||||||
主題Scheme | Other | |||||
主題 | deuterium | |||||
キーワード | ||||||
主題Scheme | Other | |||||
主題 | desorption | |||||
キーワード | ||||||
主題Scheme | Other | |||||
主題 | surface chemistry | |||||
キーワード | ||||||
主題Scheme | Other | |||||
主題 | reaction kinetics | |||||
キーワード | ||||||
主題Scheme | Other | |||||
主題 | otential energy surfaces | |||||
キーワード | ||||||
主題Scheme | Other | |||||
主題 | bonds (chemical) | |||||
出版タイプ | ||||||
出版タイプ | VoR | |||||
出版タイプResource | http://purl.org/coar/version/c_970fb48d4fbd8a85 | |||||
査読の有無 | ||||||
値 | yes | |||||
著者別名 |